Origins of “unusual” surface ozone behavior in April’2019
Abstract
The unusual behavior of surface ozone revealed in April’19 over some Belarusian cities has been analyzed. Here, the first and third decades of the month were featured by a high amplitude of the diurnal ozone course, yet, in the second decade, its sharp decrease was observed. Among possible reasons for this occurrence, one has treated changes in aerosol amount, varying meteorological conditions and levels of anthropogenic air pollution in cities. The results of the analysis indicate that the main cause of the strange behavior of surface ozone was a decrease in the vertical stability of the atmosphere leading to a more intense dispersion of pollutants and, thus, to a decrease in their concentrations in surface air. This contributed to the inhibition of the processes of surface ozone generation and destruction.
About the Authors
V. V. BozhkovaBelarus
L. M. Bolotsko
Belarus
A. M. Liudchik
Belarus
N. S. Miatelskaya
Belarus
S. D. Umreiko
Belarus
A. P. Chaikovsky
Belarus
References
1. AERONET [Electronic resource]. – Mode of access: https://aeronet.gsfc.nasa.gov. – Date of access: 07.06.2019.
2. Marathe, S. A. Multiple Regression Analysis of Ground level Ozone and its Precursor Pollutants in Coastal Mega City of Mumbai, India / S. A. Marathe, S. Murthy, N. Gosawi, M. Herlekar // MOJ Eco Environ Sci. – 2017. – Vol. 2, N 6: 00041. DOI: 10.15406/mojes.2017.02.00041
3. FIRMS [Electronic resource]. – Mode of access: https://earthdata.nasa.gov/data/near-real-time-data/firms. – Date of access: 13.06.2019.
4. HYSPLIT [Electronic resource]. – Mode of access: https://ready.arl.noaa.gov/HYSPLIT_traj.php. – Date of access: 11.08.2019.
5. Clapp, L. J. Analysis of the relationship between ambient levels of O3, NO2 and NO as a function of NOx in the UK / L. J. Clapp, M. E. Jenkin // Atmospheric Environment. – 2001. – Vol. 35. – P. 6391–6405.
6. The role of local urban traffic and meteorological conditions in air pollution: A data-based case study in Madrid, Spain / I. Laña [et al.] // Atmospheric Environment. – 2016. – Vol. 145. – P. 424‒438. http://doi.org/10.1016/j.atmosenv.2016.09.052
7. Finardi, S. Systematic analysis of meteorological conditions causing severe urban air pollution episodes in the Central Po valley / S. Finardi, U. Pellegrini // In: Institut für Meteorologie und Klimaforschung, Proceedings of the 9th Int. Conf. on Harmonisation within Atmospheric Dispersion Modelling for Regulatory Purposes, Garmisch-Partenkirchen (Germany). – 2004. – P. 250–254.
8. Verma, S. S. Effect of Meteorological Conditions on Air Pollution of Surat City / S. S. Verma, B. Desai // Journal of International Environmental Application & Science. – 2008. – Vol. 3, N 5. – P. 358–367.
9. Суточный ход концентраций загрязняющих веществ в атмосферном воздухе городов Беларуси / В. В. Божкова [и др.] // Природные ресурсы. – 2018. – № 2. – С. 79 – 87.
10. Sillman, S. Tropospheric ozone, smog and ozone-NOx-VOC sensitivity / S. Sillman // Treatise on Geochemistry. – 2003. – Vol. 9. – P. 407‒431. https://doi.org/10.1016/B0-08-043751-6/09053-8
11. Avino, P. Mechanism of smog photochemical formation in the urban area of Rome / In: Zerefos, C. S. (Ed.), Proceedings of the Quadrennial Ozone Symposium, Kos (Greece). – 2004. – P. 936–937.
12. Analysis of the Relationship between O3, NO and NO2 in Tianjin, China / S. Han [et al.] // Aerosol and Air Quality Research. – 2011. – Vol. 11. – P. 128–139. doi: 10.4209/aaqr.2010.07
13. GEOS-Chem Model [Electronic resource]. – Mode of access: http://acmg.seas.harvard.edu/geos
14. Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation / I. Bey [et al.] // J. Geophys. Res. – 2001. – Vol. 106. – P. 23073–23096.
15. GEOS-5 system [Electronic resource]. – Mode of access: http://gmao.gsfc.nasa.gov/systems/geos5/
16. GEOS-Chem – HEMCO [Electronic resource]. – Mode of access: http://wiki.seas.harvard.edu/geos-chem/index.php/ HEMCO
17. A Community Emissions Data System (CEDS) for Historical Emissions // Global Joint Change Research Institute [Electronic resource]. – Mode of access: http://www.globalchange.umd.edu/ceds/
18. POET, a database of surface emissions of ozone precursors [Electronic resource]. – Mode of access: http://www.aero. jussieu.fr/projet/ACCENT/POET.php
19. Stettler, M. E. J. Air quality and public health impacts of UK airports. Part I: Emissions / M. E. J. Stettler, S. Eastham, S. R. H. Barrett // Atmos. Environ. – 2011. – Vol. 45. – P. 5415–5424. doi:10.1016/j.atmosenv.2011.07.012
20. Revisiting global fossil fuel and biofuel emissions of ethane / Z. A. Tzompa-Sosa [et al.] // J. G. R. Atmosphere. – 2017. – Vol. 122. – P. 2493–2512. doi.org/10.1002/2016JD025767
21. The global budget of ethane and regional constraints on U.S. sources / Y. Xiao [et al.] // J. Geophys. Res. – 2008. – Vol. 113. D21306, doi:10.1029/2007JD009415
22. Yevich, R. An assesment of biofuel use and burning of agricultural waste in the developing world / R. Yevich, J. A. Logan // Global Biogeochem. Cycles. – 2003. – Vol. 17. – Р. 1095. doi:10.1029/2002GB001952.
23. Historical emissions of black and organic carbon aerosol from energy-related combustion, 1850–2000 / T. C. Bond [et al.] // Global Biogeochem. Cycles. – 2007. – Vol. 21. – GB2018. doi: 10.1029/2006GB002840
24. GFED – Global Fire Emissions Database [Electronic resource]. – Mode of access: http://www.globalfiredata.org
25. Статистическая оценка антропогенного воздействия на приземный озон / А. М. Людчик [и др.] // Природные ресурсы. – 2015. – № 1. – С. 95–105.
26. Климатическая норма приземного озона в чистой атмосфере Беларуси / В. В. Божкова [и др.] // Природные ресурсы. – 2019. – № 2. – С. 98–107.
27. Божкова, В. В. Флуктуации поля приземного озона в Беларуси, обусловленные метеорологическими условиями и антропогенным загрязнением воздуха / В. В. Божкова, А. М. Людчик, Е. А. Мельник // Природные ресурсы. – 2020. – № 1. – С. 80–91.
Review
For citations:
Bozhkova V.V., Bolotsko L.M., Liudchik A.M., Miatelskaya N.S., Umreiko S.D., Chaikovsky A.P. Origins of “unusual” surface ozone behavior in April’2019. Natural resources. 2020;(2):94-103. (In Russ.)